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JAEA Reports

Conceptual study of Post Irradiation Examination (PIE) Facility at J-PARC

Saito, Shigeru; Meigo, Shinichiro; Makimura, Shunsuke*; Hirano, Yukinori*; Tsutsumi, Kazuyoshi*; Maekawa, Fujio

JAEA-Technology 2023-025, 48 Pages, 2024/03

JAEA-Technology-2023-025.pdf:3.11MB

JAEA has been developing Accelerator-Driven Systems (ADS) for research and development of nuclear transmutation using accelerators in order to reduce the volume and hazardousness of high-level radioactive waste generated by nuclear power plants. In order to prepare the material irradiation database necessary for the design of ADS and to study the irradiation effects in Lead-Bismuth Eutectic (LBE) alloys, a proton irradiation facility is under consideration at J-PARC. In this proton irradiation facility, 250 kW proton beams will be injected into the LBE spallation target, and irradiation tests under LBE flow will be performed for candidate structural materials for ADS. Furthermore, semiconductor soft-error tests, medical RI production, and proton beam applications will be performed. Among these, Post Irradiation Examination (PIE) of irradiated samples and RI separation and purification will be carried out in the PIE facility to be constructed near the proton irradiation facility. In this PIE facility, PIE of the equipment and samples irradiated in other facilities in J-PARC will also be performed. This report describes the conceptual study of the PIE facility, including the items to be tested, the test flow, the facilities, the test equipment, etc., and the proposed layout of the facility.

Journal Articles

Neutron-production double-differential cross sections of $$^{rm nat}$$Pb and $$^{209}$$Bi in proton-induced reactions near 100 MeV

Iwamoto, Hiroki; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Ishi, Yoshihiro*; Uesugi, Tomonori*; Yashima, Hiroshi*; Nishio, Katsuhisa; Sugihara, Kenta*; $c{C}$elik, Y.*; et al.

Nuclear Instruments and Methods in Physics Research B, 544, p.165107_1 - 165107_15, 2023/11

 Times Cited Count:0 Percentile:0.02(Instruments & Instrumentation)

The lack of double-differential cross-section (DDX) data for neutron production below the incident proton energy of 200 MeV hinders the validation of spallation models in technical applications, such as research and development of accelerator-driven systems (ADSs). The present study aims to obtain experimental DDX data for ADS spallation target materials in this energy region and identify issues related to the spallation models by comparing them with the analytical predictions. The DDXs for the ($$p, xn$$) reactions of $$^{rm nat}$$Pb and $$^{209}$$Bi in the 100-MeV region were measured over an angular range of 30$$^{circ}$$ to 150$$^{circ}$$ using the time-of-flight method. The measurements were conducted at Kyoto University utilizing the FFAG accelerator. The DDXs obtained were compared with calculation results from Monte Carlo-based spallation models and the evaluated nuclear data library, JENDL-5. Comparison between the measured DDX and analytical values based on the spallation models and evaluated nuclear data library indicated that, in general, the CEM03.03 model demonstrated the closest match to the experimental values. Additionally, the comparison highlighted several issues that need to be addressed in order to improve the reproducibility of the proton-induced neutron-production DDX in the 100 MeV region by these spallation models and evaluated nuclear data library.

Journal Articles

Beam separation experiment with prototype non-destructive electrostatic septum and study for device improvement

Nagayama, Shota; Harada, Hiroyuki; Shimogawa, Tetsushi*; Sato, Atsushi*; Yamada, Ippei; Chimura, Motoki; Kojima, Kunihiro; Yamamoto, Kazami; Kinsho, Michikazu

Proceedings of 20th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.526 - 530, 2023/11

We have been developing "Non-destructive electrostatic septum" for a slow extraction. This septum has multiple electrodes placed around the region without the beam hitting and separate the beam by its electric field. To evaluate its electric field, we have built a prototype septum and a test machine, which consists of an electron gun and monitors. This test machine can measure the electric field indirectly by using a narrow electron beam. The experiment results of prototype septum is good agreement with the calculation one. However, this electric field distribution is not enough to separate the beam. A step function-like electric field distribution is ideal for the beam separation with minimal negative effect on the beam. We have studied to improve the electrode configuration to match the beam shape. In this paper, we present the result of the electric field measurements and the septum improvement. Additionally, we describe the future plan of this development.

Journal Articles

Development of a single-ended magnetic alloy loaded cavity in the Japan Proton Accelerator Research Complex rapid cycling synchrotron

Yamamoto, Masanobu; Nomura, Masahiro; Okita, Hidefumi; Shimada, Taihei; Tamura, Fumihiko; Hara, Keigo*; Hasegawa, Katsushi*; Omori, Chihiro*; Sugiyama, Yasuyuki*; Yoshii, Masahito*

Progress of Theoretical and Experimental Physics (Internet), 2023(7), p.073G01_1 - 073G01_16, 2023/07

 Times Cited Count:0 Percentile:0.01(Physics, Multidisciplinary)

The Japan Proton Accelerator Research Complex (J-PARC) Rapid Cycling Synchrotron (RCS) employs Magnetic Alloy (MA) loaded cavities. We realize multi-harmonic rf driving and beam loading compensation owing to the broadband characteristics of the MA. The currently installed cavity is the conventional type one which is designed to be driven by tube amplifiers in a push-pull operation. The push-pull operation has some advantages, i.e., suppressing a higher harmonic distortion without the beam acceleration and shortening the cavity length. However, a disadvantage arises at the high intensity beam acceleration where the multi-harmonic rf driving causes a severe imbalance of the anode voltage swing and restricts the tube operation. Although we have achieved an acceleration for the design beam power of 1 MW, the imbalance becomes an issue to further increase the beam power. We have developed a single-ended MA cavity to avoid such difficulty. The cavity has no tube imbalance intrinsically and it is found that the power consumption to drive the cavity can be reduced compared with the conventional one.

Journal Articles

Measurement of 107-MeV proton-induced double-differential thick target neutron yields for Fe, Pb, and Bi using a fixed-field alternating gradient accelerator at Kyoto University

Iwamoto, Hiroki; Nakano, Keita; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Sugihara, Kenta; Nishio, Katsuhisa; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; et al.

Journal of Nuclear Science and Technology, 60(4), p.435 - 449, 2023/04

 Times Cited Count:3 Percentile:68.71(Nuclear Science & Technology)

Double-differential thick target neutron yields (TTNYs) for Fe, Pb, and Bi targets induced by 107-MeV protons were measured using the fixed-field alternating gradient accelerator at Kyoto University for research and development of accelerator-driven systems (ADSs) and fundamental ADS reactor physics research at the Kyoto University Critical Assembly (KUCA). Note that TTNYs were obtained with the time-of-flight method using a neutron detector system comprising eight neutron detectors; each detector has a small NE213 liquid organic scintillator and photomultiplier tube. The TTNYs obtained were compared with calculation results using Monte Carlo-based spallation models (i.e., INCL4.6/GEM, Bertini/GEM, JQMD/GEM, and JQMD/SMM/GEM) and the evaluated high-energy nuclear data library, i.e., JENDL-4.0/HE, implemented in the particle and heavy iontransport code system (PHITS). All models, including JENDL-4.0/HE, failed to predict high-energy peaks at a detector angle of 5$$^{circ}$$. Comparing the energy- and angle-integrated spallation neutron yields at energies of $$le$$20 MeV estimated using the measured TTNYs and the PHITS indicated that INCL4.6/GEM would be suitable for the Monte Carlo transport simulation of ADS reactor physics experiments at the KUCA.

JAEA Reports

Development of bearing units used in the rotating shaft system for power generation in the JAEA-Tokai Tandem accelerator

Otokawa, Yoshinori; Matsuda, Makoto; Abe, Shinichi

JAEA-Technology 2022-037, 23 Pages, 2023/03

JAEA-Technology-2022-037.pdf:5.38MB

Bearing units of rotating shaft system for power generation in the JAEA-Tokai Tandem accelerator had a short operating life from the beginning of the accelerator installation, and even after replacing the bearing unit, early failures often occurred. Therefore, the quantity and frequency of replacement are large, and a lot of time is spent in regular maintenance performed by opening the accelerator pressure vessel, and solving this problem has been a long-standing concern. As a result of considering the cause of this early failure, it was considered that the load caused by parallel, angular, and axial misalignment of the upper and lower bearing units was the cause. In order to solve this problem, we have developed a bearing unit having metal disc-spring couplings in the upper and lower flanges to allow for parallel, angular, and axial misalignment of bearing units. As a result, it is now possible to allow variations in the distance between castings and parallel, angular, and axial misalignment of the upper and lower bearing units. By installing the developed new bearing unit on the rotating shaft system and making improvements while continuing to use it in actual operation, we succeeded in reducing the early failure and extending the operating life by more than double. With this development, the maintenance time has been reduced to one week by reducing the number of replacing the bearing unit. In addition, we have realized one regular maintenance that was carried out about three times a year, and as a benefit, we were able to reduce the amount of sulfur hexafluoride (SF$$_{6}$$) gas, which is a greenhouse gas, to about 33$$sim$$50% per year. We describe about development of new bearing units and these maintenance status from 2006 to 2020.

JAEA Reports

Development of freezed seal valve by using test stand for LBE technology

Saito, Shigeru; Yamaguchi, Kazushi*; Yoshimoto, Hidemitsu*; Obayashi, Hironari; Sasa, Toshinobu

JAEA-Technology 2022-032, 51 Pages, 2023/03

JAEA-Technology-2022-032.pdf:4.51MB

In the Accelerator Driven System (ADS) being studied by the Japan Atomic Energy Agency (JAEA) for transmutation of long-lived radioactive waste, lead-bismuth eutectic alloy (LBE) is used as a spallation target and subcritical core coolant. A proton irradiation facility in J-PARC is considered to prepare a material irradiation database for ADS development. The proton irradiation facility is equipped with an LBE loop, which enables material irradiation tests in spallation environment under flowing LBE condition. The slow leakage of LBE is one of critical issue to use LBE safety. The slow leakage is caused by the biting slag and/or other materials at valve seal of drain valve. To solve this problem, JAEA examined the application of freeze-seal valve (FSV), which seal the piping by freezing LBE in specific position. Water-cooled and air-cooled freeze-seal valve test modules were fabricated, installed in the test section of the existing test stand for LBE technology development, and tested to confirm their operation and performance. As a result of the tests, it was confirmed that the water-cooled FSV test module worked well along to the design values. This report describes the outline and details of the test stand for LBE technology and each FSV test module, as well as the results of operation and performance verification tests.

JAEA Reports

Proceedings of the 34th Meeting for Tandem Accelerators and their Associated Technologies

Kabumoto, Hiroshi; Nakagawa, Sohei; Matsuda, Makoto

JAEA-Conf 2022-002, 146 Pages, 2023/03

JAEA-Conf-2022-002.pdf:9.89MB

"The 34th Meeting for Tandem Accelerators and their Associated Technologies" was held on July 21-22, 2022 organized by Nuclear Science Research Institute of the Japan Atomic Energy Agency. This meeting was held only on-line for preventing the spread of COVID-19 infection. The purpose of this meeting is contribution of development for related technology and of management of facilities through exchange of information among the researchers and engineers using and operating electrostatics accelerator facilities like tandem accelerators. There were 25 presentations which contains current status report of facility, technical development of accelerator, research of application. The total number of participants was a hundred, from 26 universities, research organizations and industries. This meeting consisted of only oral session, a poster session was not carried out because of on-line meeting. This proceeding compiles the contents of report papers in the meeting.

Journal Articles

Toward nuclear transmutation

Maekawa, Fujio

Ryoshi Bimu Kagaku No Kiso To Oyo; NSA/Commentaries, No.27, p.15 - 25, 2023/03

The nuclear transmutation technology that is one of the most beneficial industrial applications of quantum beams to humankind is explained.

Journal Articles

Present status of JAEA-Tokai tandem accelerator

Kabumoto, Hiroshi; Matsuda, Makoto; Nakamura, Masahiko; Ishizaki, Nobuhiro; Kutsukake, Kenichi; Otokawa, Yoshinori; Asozu, Takuhiro; Matsui, Yutaka; Nakagawa, Sohei; Abe, Shinichi

Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1109 - 1113, 2023/01

no abstracts in English

Journal Articles

Reports of electro-polishing implementation for quarter-wave resonators, 2

Nii, Keisuke*; Ida, Yoshiaki*; Ueda, Hideki*; Yamaguchi, Takanori*; Kabumoto, Hiroshi; Kamiya, Junichiro; Kondo, Yasuhiro; Tamura, Jun; Harada, Hiroyuki; Matsui, Yutaka; et al.

Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.601 - 604, 2023/01

no abstracts in English

Journal Articles

Study of non-destructive slow beam extraction method in particle accelerator

Nagayama, Shota; Harada, Hiroyuki; Shimogawa, Tetsushi*; Yamada, Ippei; Chimura, Motoki; Yamamoto, Kazami; Kinsho, Michikazu

Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.503 - 507, 2023/01

Synchrotron accelerators realize physics experiments and radiation cancer treatment using the slow extraction technique, in which beams are stored in the ring and gradually delivered. We have devised and are currently developing a "non-destructive electrostatic septum" based on a new method, which in principle cannot be solved by conventional methods and is a cause of equipment failure and output limitation. It is ideal to generate a force distribution similar to a staircase function with discontinuous gaps at the boundary. In this presentation, we will show the calculation method for optimizing the electrode and wire configuration to generate a Lorentz force with a distribution similar to a staircase function in vacuum, and the calculation results of the beam breakup due to the generated Lorentz force. The compact proof-of-principle machine developed for the ongoing demonstration of this method will also be introduced.

Journal Articles

Development of an ion funnel reaction cell for suppression of isobaric interference in chrorin-36 dating

Jinno, Satoshi; Fujita, Natsuko; Tanuma, Hajime*

Dai-23-Kai AMS Shimpojiumu Hokokushu, p.89 - 92, 2022/12

The measurement of chlorine-36 ($$^{36}$$Cl) in AMS, which is important for the dating of saline groundwater, is more difficult than other nuclides due to the isobaric interference by sulfur-36 ($$^{36}$$S). In general, acceleration voltages of 6 MV or higher are required to separate $$^{36}$$Cl and $$^{36}$$S. Therefore, this study aims to develop an ion funnel reaction cell and incorporate it into the low energy side of JAEA-AMS-TONO-5MV to selectively suppress $$^{36}$$S.

Journal Articles

Frontiers of studies utilizing accelerator mass spectrometry in geoscience

Honda, Maki

Journal of the Mass Spectrometry Society of Japan, 70(4), p.282 - 283, 2022/12

The development of measurement and chemical separation techniques in the accelerator mass spectrometry (AMS) method has enabled highly sensitive analysis of $$^{244}$$Pu (half-life 8.1$$times$$10$$^{7}$$ years), $$^{60}$$Fe (half-life 2.62$$times$$10$$^{6}$$ years), and $$^{90}$$Sr (half-life 28.9 years) in AMS. For example, the study analyzing $$^{244}$$Pu in ferromanganese crust samples successfully quantified $$^{244}$$Pu from outside the solar system, which had been hidden by $$^{244}$$Pu from nuclear tests. Furthermore, the research has revealed that $$^{244}$$Pu is produced in neutron star mergers, etc., leading to unraveling the production sites where the heavy elements originate. This topic highlights the frontline of studies on $$^{244}$$Pu, $$^{60}$$Fe, and $$^{90}$$Sr utilizing AMS.

Journal Articles

Challenging studies by accelerator mass spectrometry for the development of environmental radiology; Status report on the analysis of $$^{90}$$Sr and $$^{135}$$Cs by AMS

Honda, Maki; Martschini, M.*; Wieser, A.*; Marchhart, O.*; Lachner, J.*; Priller, A.*; Steier, P.*; Golser, R.*; Sakaguchi, Aya*

JAEA-Conf 2022-001, p.85 - 90, 2022/11

Accelerator mass spectrometry (AMS) is an analytical method that combines mass spectrometry with a tandem accelerator, which has been used mainly in nuclear physics experiments. AMS is used to measure radionuclides with half-lives of 10$$^{3}$$-10$$^{8}$$ years. For radionuclides with half-lives of this order, the method of measuring their mass is 10$$^{3}$$-10$$^{6}$$ times more sensitive than measuring their activity. Because of this advantage, AMS has been widely applied in Earth and planetary sciences, atomic energy research, and other fields. Among the various studies, Wallner et al. (2021, 2016) have achieved excellent work in Earth and planetary sciences. For example, they have attained the ultra-sensitive analysis of $$^{60}$$Fe and $$^{244}$$Pu in environmental samples. These are radionuclides produced by rapid-neutron-capture (r-process) nucleosynthesis. Our recent work shows that a new AMS system (VERA, University of Vienna), which combines laser isobaric separation and a typical AMS system, has been successfully applied to the ultra-sensitive determination of $$^{90}$$Sr and $$^{135}$$Cs in environment. For $$^{90}$$Sr in environmental samples, the $$beta$$-ray measurement by the milking of the daughter nuclide $$^{90}$$Y is still the principal method, which takes 3-6 weeks. The new AMS method has a detection limit of $$<$$ 0.1 mBq, which is comparable to that of $$beta$$-ray measurement, with a more straightforward chemical treatment than $$beta$$-measurement. Our achievement demonstrates that AMS can be a practical new method for determining $$^{90}$$Sr in the environment.

Journal Articles

Paper award of Atomic Energy Society of Japan in 2021; JENDL/DEU-2020: deuteron nuclear data library for design studies of accelerator-based neutron sources

Nakayama, Shinsuke

Kaku Deta Nyusu (Internet), (133), p.88 - 99, 2022/10

The content of the paper that received the Paper Award of Atomic Energy Society of Japan in 2021 is outlined. Although the use of deuteron accelerator-based neutron sources has been proposed in various fields, deuteron nuclear database accurate enough to be applied to the design study of such neutron sources had not been developed. Under these situations, we had developed a deuteron nuclear database, JENDL/DEU-2020. It contains evaluated deuteron nuclear data for light nuclei ($$^{6,7}$$Li, $$^{9}$$Be, $$^{12,13}$$C), which are candidates for deuteron beam irradiation targets of the neutron sources. Evaluation of JENDL/DEU-2020 was performed by using the code system DEURACS with further modifications. In order to validate the accuracy of the database, simulations using the particle transport code were performed under various conditions with different target nuclides and incident deuteron energies, and the results were compared with the available experimental data. As a result, it was found that JENDL/DEU-2020 significantly improves the prediction accuracy of experimental data under a wider range of conditions than other nuclear reaction databases or the nuclear reaction models implemented in transport calculation codes.

Journal Articles

Development of combined-function multipole permanent magnet for high-intensity beam transportation

Fuwa, Yasuhiro; Takayanagi, Tomohiro; Iwashita, Yoshihisa*

IEEE Transactions on Applied Superconductivity, 32(6), p.4006705_1 - 4006705_5, 2022/09

 Times Cited Count:0 Percentile:0(Engineering, Electrical & Electronic)

Space charge compensation technique using multipole magnetic field components has been proposed to transport high intensity beam in the J-PARC linac. In order to realize this compensation technique, a compact size permanent hybrid multi-pole magnet would be suitable. A magnet system for the simultaneous production of quadrupole and adjustable octupole components using permanent magnet materials and have manufactured a first model of the magnet systems.

Journal Articles

Design of beam focusing system with permanent magnet for J-PARC LINAC MEBT1

Fuwa, Yasuhiro; Moriya, Katsuhiro; Takayanagi, Tomohiro

Proceedings of 31st International Linear Accelerator Conference (LINAC 2022) (Internet), p.364 - 367, 2022/09

MEBT1 (Medium Energy Beam Transport 1) of the J-PARC LINAC is a 3 MeV beam transport system located between the RFQ (Radio Frequency Quadrupole) and DTL (Drift Tube Linac). In the MEBT1, the beam-optical matching for injection into DLT and chopping for injection into acceleration phase of 3 GeV synchrotron, located downstream to the LINAC, are performed. The characteristics of MEBT1 are an important factor in determining the beam quality in the J-PARC accelerator facility. To achieve beam power of 1 MW and beyond, improving the stability and reliability of MEBT1 is an important development issue. The application of permanent magnets to the beam focusing system to the MEBT1 is under consideration to achieve improved stability and reliability. In this presentation, we report the design of focusing magnets using permanent magnet material and the results of the lattice study of MEBT1 with permanent magnets.

Journal Articles

Properties of praseodymium permanent magnet for cryogenic hybrid magnet

Fuwa, Yasuhiro; Iwashita, Yoshihisa*; Kondo, Akihiro*

IEEE Transactions on Applied Superconductivity, 32(6), p.4007304_1 - 4007304_4, 2022/06

 Times Cited Count:0 Percentile:0(Engineering, Electrical & Electronic)

High-field magnets are often demanded advanced scientific studies. Although a hybrid coil design comprising Nb-Ti, Nb$$_{3}$$Sn, and HTS (High-Temperature Superconductors) are potential candidates for such application, the costs of Nb$$_{3}$$Sn and HTS are expensive compared with Nb-Ti. By generating an additional field of about 1 T by permanent magnets, the required amounts of superconducting material may be reduced. Magnetic properties of some magnetic materials have been studied by other works at temperatures as low as 100 K. The remanent field of conventional NdFeB magnets decreases at 100 K due to spin reorientation. PrFeB magnets consisting of praseodymium (Pr) instead of neodymium (Nd) do not show such degradation and the coercivity of PrFeB at 100 K is 7 T. In this study, the B-H curve, as a primary magnetic property, of a PrFeB magnet sample was measured in the temperature range down to 4 K. As a result, no decrease in magnetization of the praseodymium magnets, and the coercivity was 10 T.

Journal Articles

Beam emittance growth due to the strong space-charge field at low energy of a high-intensity ion linac and its mitigation using an octupole magnetic field

Chimura, Motoki; Harada, Hiroyuki; Kinsho, Michikazu

Progress of Theoretical and Experimental Physics (Internet), 2022(6), p.063G01_1 - 063G01_26, 2022/06

 Times Cited Count:1 Percentile:28(Physics, Multidisciplinary)

In the low-energy region of a high-intensity ion linac, a strong space-charge field causes a rapid beam emittance growth over a short distance of only few meters. The beam emittance growth leads to a beam loss and the machine activation raising a serious issue for regular maintenance of the accelerator component and beam power ramp up. In this work, we studied the mechanism of beam emittance growth due to the space-charge field based on three-dimensional particle-tracking simulation and theoretical considerations. Numerical simulations done for the high-intensity linac at J-PARC shows that the nonlinear terms in the space-charge field directly cause a beam emittance growth and beam halo formation. Then, we also propose a method to mitigate the beam emittance growth by using an octupole magnetic field, which arises as one of the nonlinear terms in the space-charge field. By applying this method in the simulation, we have succeeded mitigating the beam emittance growth.

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